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可持续发展 4

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Biodiesel production from waste frying oil in sub- and supercritical methanol on a zeolite Y solid acid

Jorge MEDINA-VALTIERRA, Jorge RAMIREZ-ORTIZ

《化学科学与工程前沿（英文）》 2013年 第7卷 第4期   页码 401-407 doi: 10.1007/s11705-013-1354-1

摘要： Waste frying oil (WFO) is a very important feedstock for obtaining biodiesel at low cost and using WFO in transesterification reactions to produce biodiesel helps eliminate local environmental problems. In this study biodiesel was produced from WFO in sub- and super-critical methanol on a zeolite Y solid acid catalyst. The procedure was optimized using a design of experiments by varying the methanol to WFO molar ratio, the reaction temperature, and the amount of catalyst. Typical biodiesel yields varied from 83 to nearly 100% with methyl esters content ranging from 1.41–1.66 mol·L and typical dynamic viscosities of 22.1-8.2 cP. Gas chromatography was used to determine the molecular composition of the biodiesel. The reaction products contained over 82 wt-% methyl esters, 4.2 wt-% free acids, 13.5 wt-% monoglycerides, and 0.3 wt-% diglycerides. The transesterification of WFO with methanol around its critical temperature combined with a zeolite Y as an acid catalyst is an efficient approach for the production of biodiesel with acceptable yields.

关键词： biodiesel     methanol     critical temperature     waste frying oil     zeolite Y    

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engine performance, emission and combustion characteristics fueled with diesel-like fuel produced from wasteengine oil and waste plastics

V. Edwin Geo, Ankit Sonthalia, Fethi Aloui, Femilda Josephin J. S.

《环境科学与工程前沿（英文）》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1063-6

摘要：

To derive liquid fuel from waste engine oil and plastics thorough pyrolysis process

To make equal blend of waste engine oil and plastics with diesel fuel

To find the suitability of fuel from waste in diesel engine through performance, emission and combustion characteristics

关键词： Waste engine oil     Waste plastic oil     Diesel fuel     Pyrolysis     Compression ignition engine    

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Highly hydrophobic oil−water separation membrane: reutilization of waste reverse osmosis membrane

《化学科学与工程前沿（英文）》 2023年 第17卷 第10期   页码 1606-1615 doi: 10.1007/s11705-022-2200-0

摘要： The increasing applications of seawater desalination technology have led to the wide usage of polyamide reverse osmosis membranes, resulting in a large number of wasted reverse osmosis membranes. In this work, the base nonwoven layer of the wasted reverse osmosis membrane was successfully modified into the hydrophobic membrane via surface deposition strategy including TiO2 and 1H,1H,2H,2H-perfluorooctyltrichlorosilane (PFOTS), respectively. Various techniques were applied to characterize the obtained membranes, which were then used to separate the oil–water system. The optimally modified membrane displayed good hydrophobicity with a contact angle of 135.2° ± 0.3°, and its oil–water separation performance was as high as 97.8%. After 20 recycle tests, the oil–water separation performance remained more than 96%, which was attributed to the film adhesion of the anchored TiO2 and PFOTS layer on the surface. This work might provide a new avenue for recycling the wasted reverse osmosis membrane used in oily wastewater purification.

关键词： oil–water separation     wasted reverse osmosis membrane     hydrophobic modification    

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MILP synthesis of separation processes for waste oil-in-water emulsions treatment

Zorka N. Pintarič,Gorazd P. Škof,Zdravko Kravanja

《化学科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 120-130 doi: 10.1007/s11705-016-1559-1

摘要： This paper presents a novel synthesis method for designing integrated processes for oil-in-water (O/W) emulsions treatment. General superstructure involving alternative separation technologies is developed and modelled as a mixed integer linear programming (MILP) model for maximum annual profit. Separation processes in the superstructure are divided into three main sections of which the pretreatment and final treatment are limited to the selection of one alternative (or bypass) only, while within the intermediate section various combinations of different technologies in series can be selected. Integrated processes composed of selected separation techniques for given ranges of input chemical oxygen demand (COD) can be proposed by applying parametric analyses within the superstructure approach. This approach has been applied to an existing industrial case study for deriving optimal combinations of technologies for treating diverse oil-in-water emulsions within the range of input COD values between 1000 mg?L and 145000 mg?L . The optimal solution represents a flexible and profitable process for reducing the COD values below maximal allowable limits for discharging effluent into surface water.

关键词： oil-in-water emulsion     chemical oxygen demand     superstructure     process synthesis     MILP    

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Metakaolinite as a catalyst for biodiesel production from waste cooking oil

Jorge RAMIREZ-ORTIZ, Merced MARTINEZ, Horacio FLORES

《化学科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 403-409 doi: 10.1007/s11705-012-1224-2

摘要： The use of metakaolinite as a catalyst in the transesterification reaction of waste cooking oil with methanol to obtain fatty acid methyl esters (biodiesel) was studied. Kaolinite was thermally activated by dehydroxylation to obtain the metakaolinite phase. Metakaolinite samples were characterized using X-ray diffraction, N adsorption-desorption, simultaneous thermo-gravimetric analyse/differential scanning calorimetry (TGA/DSC) experiments on the thermal decomposition of kaolinite and Fourier-transform infrared spectrometer (FTIR) analysis. Parameters related to the transesterification reaction, including temperature, time, the amount of catalyst and the molar ratio of waste cooking oil to methanol, were also investigated. The transesterification reaction produced biodiesel in a maximum yield of 95% under the following conditions: metakaolinite, 5 wt-% (relative to oil); molar ratio of oil to methanol, 1∶23; reaction temperature, 160°C; reaction time, 4 h. After eight consecutive reaction cycles, the metakaolinite can be recovered and reused after being washed and dried. The biodiesel thus obtained exhibited a viscosity of 5.4?mm ?s and a density of 900.1 kg?m . The results showed that metakaolinite is a prominent, inexpensive, reusable and thermally stable catalyst for the transesterification of waste cooking oil.

关键词： biodiesel     metakaolinite     transesterification     waste cooking oil    

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我国生物柴油产业发展的探讨

闵恩泽,杜泽学

《中国工程科学》 2010年 第12卷 第2期   页码 11-15

摘要：

介绍了美国、欧盟等和我国生物柴油产业发展的最新进展，包括产能、标准和政策等。从原料供应和生产经济性角度分析了我国生物柴油产业发展面临的困境，并建议采用废弃油脂作为起点，推动我国生物柴油产业发展，特别是要用生物柴油（脂肪酸甲酯）和甘油来生产高附加值的化工产品，大幅度提高利润。

关键词： 生物柴油     废弃油脂     经济可行性     化工产品    

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Integrated approach to winery waste: waste generation and data consolidation

Margarida OLIVEIRA,Elizabeth DUARTE

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 168-176 doi: 10.1007/s11783-014-0693-6

摘要： The winemaking process involves the generation of a significant amount of waste and wastewater. These residues should be addressed for recycling or treatment before being returned to environment. As each winery is unique in waste generation and disposal, plans for environmentally friendly waste management are not universal and should be tested for their effectiveness. In this study, a diagnostic was made during three years, in different wineries, throughout Portugal, in order to quantify and characterize the waste and the wastewater produced. The results showed that solid waste and wastewater are mainly produced during the harvest period, corresponding to 74% and 87%, respectively. One ton of processed grape approximately produce 0.13 t marc, 0.06 t lees, 0.03 t of stalks and 1.65 m of wastewater. No significant differences ( ≤0.05) were observed for grape marc, lees and wastewater ratios, between years or wineries. With respect to the stalk ratio, there was no effect of year but the winery significantly affected this ratio ( ≤0.05). During the study period the treated wastewater, since diluted, revealed suitable characteristics for irrigation representing an additional source of water. In this regard, the data acquisition and consolidation ensure the transfer of information and experience which constitute an essential step in a support decision tool design.

关键词： waste management     wastewater reuse     winery wastewater    

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The road to sustainable use and waste management of plastics in Portugal

《环境科学与工程前沿（英文）》 2022年 第16卷 第1期   页码 5-5 doi: 10.1007/s11783-021-1439-x

摘要：

• Portugal recycles 34% of the 40 kg/hab year of plastic packaging waste.

关键词： Single-use plastics     Plastic packaging     Plastic waste     Waste management     Waste shipment     Lightweight plastic bags    

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VALORIZATION OF LIVESTOCK WASTE AND CARBON NEUTRALITY

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 333-340 doi: 10.15302/J-FASE-2023513

摘要： VALORIZATION OF LIVESTOCK WASTE AND CARBON NEUTRALITY

关键词： WASTE     CARBON     VALORIZATION     NEUTRALITY    

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Repercussions of COVID-19 pandemic on solid waste generation and management strategies

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1407-5

摘要：

• Implication of COVID-19 on medical waste and MSW generation is studied.

关键词： COVID-19     Medical waste     Personal protective equipment     Municipal solid waste     Waste management    

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Industrial solid waste flow analysis of eco-industrial parks: implications for sustainable waste management

Yongpeng Lü, Kai YANG, Yue CHE, Zhaoyi SHANG, Jun TAI, Yun JIAN

《环境科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 575-587 doi: 10.1007/s11783-011-0344-0

摘要： Sustainable waste management in the industrial ecology perspective brings enormous challenges to the existing methodology of waste analysis at the industrial park (IP) scale. In this study, a four-step method was proposed for industrial solid waste (ISW) flow analysis of eco-industrial parks (EIPs) and applied to two IPs in eastern China. According to a park-wide census of 619 industrial enterprises and 105 questionnaires by a survey from 2006 to 2008, the results indicated that: 1) at the enterprise scale, more than 60% of enterprises were small-ISW-generation enterprises which encountered great difficulties on effective waste management; 2) at the IP scale, though the two IPs have set up their own environmental management systems and passed the ISO 14001 certification, the efficiencies of the ISW management systems have yet to be improved in the industrial ecology perspective; and 3) at the regional scale, more than 97% of ISW flowed within the provincial region, indicating that the provincial governments prevented the wastes from flowing into their own “back yard”. Effective waste management should be placed in a broader perspective. Approaches to sustainable waste management may include wastes exchange, efficient waste and information flow, virtual EIP, waste minimization clubs and regionalization of waste management.

关键词： industrial solid waste     waste flow analysis     eco-industrial parks     sustainable waste management     “not in my back yard”    

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Biodegradation of waste refrigerator polyurethane by mealworms

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1638-8

摘要：

● Waste refrigerator polyurethane (WRPU) was ingested and biodegraded by mealworms.

关键词： Waste refrigerator polyurethane     Mealworms     Biodegradation     Carbon balance     Gut microorganism    

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Co-fermentation of waste activated sludge with food waste for short-chain fatty acids production: effect

Leiyu FENG, Yuanyuan YAN, Yinguang CHEN

《环境科学与工程前沿（英文）》 2011年 第5卷 第4期   页码 623-632 doi: 10.1007/s11783-011-0334-2

摘要： Effect of pH ranging from 4.0 to 11.0 on co-fermentation of waste activated sludge (WAS) with food waste for short-chain fatty acids (SCFAs) production at ambient temperature was investigated in this study. Experimental results showed that the addition of food waste significantly improved the performance of WAS fermentation system, which resulted in the increases of SCFAs production and substrate reduction. The SCFAs production at pH 6.0, 7.0, 8.0, and 9.0 and fermentation time of 4 d was respectively 5022.7, 6540.5, 8236.6, and 7911.7 mg COD·L , whereas in the blank tests (no pH adjustment, pH 8.0 (blank test 1), no food waste addition, pH 8.0 (blank test 2), and no WAS addition (blank test 3)) it was only 1006.9, 971.1, and 1468.5 mg COD·L , respectively. The composition of SCFAs at pH from 6.0 to 9.0 was also different from other conditions and propionic acid was the most prevalent SCFA, which was followed by acetic and n-butyric acids, while acetic acid was the top product under other conditions. At pH 8.0 a higher volatile suspended solids (VSS) reduction of 16.6% for the mixture of WAS and food waste than the sole WAS indicated a synergistic effect existing in fermentation system with WAS and food waste. The influence of pH on the variations of nutrient content was also studied during anaerobic fermentation of the mixture of WAS and food waste at different pH conditions. The release of increased with fermentation time at all pH values investigated except 4.0, 5.0 and in blank test one. The concentrations of soluble phosphorus at acidic pHs and in the blank test one were higher than those obtained at alkaline pHs. Ammonia and phosphorus need to be removed before the SCFAs-enriched fermentation liquid from WAS and food waste was used as the carbon source.

关键词： waste activated sludge (WAS)     food waste     co-fermentation     short-chain fatty acids (SCFAs)     pH     synergistic effect    

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Biodegradable, superhydrophobic walnut wood membrane for the separation of oil/water mixtures

《化学科学与工程前沿（英文）》 2022年 第16卷 第9期   页码 1377-1386 doi: 10.1007/s11705-022-2157-z

摘要： The preparation of environmentally friendly oil/water separation materials remains a great challenge. Freeze-drying of wood after lignin removal yields wood aerogels, which can be used as substrates to prepare fluorine-free environmentally friendly superhydrophobic materials, However, they are more suitable for absorption rather than filtration applications due to their poor strength. A study using cross-sections of pristine wood chips as substrates retains the original strength of wood, but the use of the cross-sectional of wood pieces limits their thickness, strength, and size. In this paper, a degradable fluorine-free superhydrophobic film (max. water contact angle of approximately 164.2°) with self-cleaning and abrasion resistance characteristics was prepared by a one-step method using pristine and activated walnut longitudinal section films as the substrate, with tetraethyl orthosilicate as a precursor and dodecyltriethoxysilane as a modifier. The tensile strength results show that superhydrophobic films with pristine or activated wood substrates maintained the strength of pristine wood and were 2.2 times stronger than the wood aerogel substrate. In addition, after cross-laminating the two samples, the films had the ability to separate oil and water by continuous filtration with high efficiency (98.5%) and flux (approximately 1.3 × 103 L∙m‒2∙h‒1). The method has potential for the large-scale fabrication of degradable superhydrophobic filtration separation membranes.

关键词： wood nanotechnology     superhydrophobic     biodegradable     surface modification     oil/water separation    

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Pyrolysis of WEEE plastics using catalysts produced from fly ash of coal gasification

Marika Benedetti, Lorenzo Cafiero, Doina De Angelis, Alessandro Dell’Era, Mauro Pasquali, Stefano Stendardo, Riccardo Tuffi, Stefano Vecchio Ciprioti

《环境科学与工程前沿（英文）》 2017年 第11卷 第5期 doi: 10.1007/s11783-017-0998-3

摘要： Catalytic pyrolysis of thermoplastics extracted from waste electrical and electronic equipment (WEEE) was investigated using various fly ash-derived catalysts. The catalysts were prepared from fly ash by a simple method that basically includes a mechanical treatment followed by an acid or a basic activation. The synthesized catalysts were characterized using various analytical techniques. The results showed that not treated fly ash (FA) is characterized by good crystallinity, which in turn is lowered by mechanical and chemical treatment (fly ash after mechanical and acid activation, FAMA) and suppressed almost entirely down to let fly ash become completely amorphous (fly ash after mechanical and basic activation FAMB). Simultaneously, the surface area resulted increased. Subsequently, FA, FAMB and FAMA were used in the pyrolysis of a WEEE plastic sample at 400°C and their performance were compared with thermal pyrolysis at the same temperature. The catalysts principally improve the light oil yield: from 59wt.% with thermal pyrolysis to 83 wt.% using FAMB. The formation of styrene in the oil is also increased: from 243 mg/g with thermal pyrolysis to 453 mg/g using FAMB. As a result, FAMB proved to be the best catalyst, thus producing also the lowest and the highest amount of char and gas, respectively.

关键词： Waste electrical and electronic equipment (WEEE) plastic mixture     Pyrolysis     Catalyst     Fly ash     Oil    

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标题 作者 时间 类型 操作

Biodiesel production from waste frying oil in sub- and supercritical methanol on a zeolite Y solid acid

Jorge MEDINA-VALTIERRA, Jorge RAMIREZ-ORTIZ

期刊论文

engine performance, emission and combustion characteristics fueled with diesel-like fuel produced from wasteengine oil and waste plastics

V. Edwin Geo, Ankit Sonthalia, Fethi Aloui, Femilda Josephin J. S.

期刊论文

Highly hydrophobic oil−water separation membrane: reutilization of waste reverse osmosis membrane

期刊论文

MILP synthesis of separation processes for waste oil-in-water emulsions treatment

Zorka N. Pintarič,Gorazd P. Škof,Zdravko Kravanja

期刊论文

Metakaolinite as a catalyst for biodiesel production from waste cooking oil

Jorge RAMIREZ-ORTIZ, Merced MARTINEZ, Horacio FLORES

期刊论文

我国生物柴油产业发展的探讨

闵恩泽,杜泽学

期刊论文

Integrated approach to winery waste: waste generation and data consolidation

Margarida OLIVEIRA,Elizabeth DUARTE

期刊论文

The road to sustainable use and waste management of plastics in Portugal

期刊论文

VALORIZATION OF LIVESTOCK WASTE AND CARBON NEUTRALITY

期刊论文

Repercussions of COVID-19 pandemic on solid waste generation and management strategies

期刊论文

Industrial solid waste flow analysis of eco-industrial parks: implications for sustainable waste management

Yongpeng Lü, Kai YANG, Yue CHE, Zhaoyi SHANG, Jun TAI, Yun JIAN

期刊论文

Biodegradation of waste refrigerator polyurethane by mealworms

期刊论文

Co-fermentation of waste activated sludge with food waste for short-chain fatty acids production: effect

Leiyu FENG, Yuanyuan YAN, Yinguang CHEN

期刊论文

Biodegradable, superhydrophobic walnut wood membrane for the separation of oil/water mixtures

期刊论文

Pyrolysis of WEEE plastics using catalysts produced from fly ash of coal gasification

Marika Benedetti, Lorenzo Cafiero, Doina De Angelis, Alessandro Dell’Era, Mauro Pasquali, Stefano Stendardo, Riccardo Tuffi, Stefano Vecchio Ciprioti

期刊论文